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Once the lending period for a Kindle Book is over, it will expire. Although you can't open an expired title, you do have to manually remove it from your device.
If you're using a Kindle reading app, Kindle Fire, or Kindle Touch, long-press a title, then choose Remove from Device. If you're using a Kindle, push to the right on the directional pad, then select Remove from Device.
Once a Kindle Book has been removed from your device, you can also remove it from 'Your Kindle Library' on the 'Manage Your Kindle' page. This removes the titles from your 'Archived' items the next time you sync.